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dc.provenanceFacultad de Ciencias Exactas y Naturales de la UBA-
dc.contributorCampo, M.G.-
dc.contributorGrigera, J.R.-
dc.creatorCampo, M.G.-
dc.creatorGrigera, J.R.-
dc.date.accessioned2018-05-04T22:02:07Z-
dc.date.accessioned2018-05-28T15:47:51Z-
dc.date.available2018-05-04T22:02:07Z-
dc.date.available2018-05-28T15:47:51Z-
dc.date.issued2005-
dc.identifier.urihttp://10.0.0.11:8080/jspui/handle/bnmm/68369-
dc.descriptionWe have studied the hydration and diffusion of the hydroxyl radical O H0 in water using classical molecular dynamics. We report the atomic radial distribution functions, hydrogen-bond distributions, angular distribution functions, and lifetimes of the hydration structures. The most frequent hydration structure in the O H0 has one water molecule bound to the O H0 oxygen (57% of the time), and one water molecule bound to the O H0 hydrogen (88% of the time). In the hydrogen bonds between the O H0 and the water that surrounds it the O H0 acts mainly as proton donor. These hydrogen bonds take place in a low percentage, indicating little adaptability of the molecule to the structure of the solvent. All hydration structures of the O H0 have shorter lifetimes than those corresponding to the hydration structures of the water molecule. The value of the diffusion coefficient of the O H0 obtained from the simulation was 7.1× 10-9 m2 s-1, which is higher than those of the water and the O H-. © 2005 American Institute of Physics.-
dc.formatapplication/pdf-
dc.languageeng-
dc.rightsinfo:eu-repo/semantics/openAccess-
dc.rightshttp://creativecommons.org/licenses/by/2.5/ar-
dc.sourceJ Chem Phys 2005;123(8)-
dc.source.urihttp://digital.bl.fcen.uba.ar/Download/paper/paper_00219606_v123_n8_p_Campo.pdf-
dc.subjectAngular distribution functions-
dc.subjectAtomic radial distribution functions-
dc.subjectHydroxyl radicals-
dc.subjectWater molecules-
dc.subjectComputer simulation-
dc.subjectDiffusion-
dc.subjectHydrogen bonds-
dc.subjectMolecular dynamics-
dc.subjectSolvents-
dc.subjectWater-
dc.subjectFree radicals-
dc.titleClassical molecular-dynamics simulation of the hydroxyl radical in water-
dc.typeinfo:eu-repo/semantics/article-
dc.typeinfo:ar-repo/semantics/artículo-
dc.typeinfo:eu-repo/semantics/publishedVersion-
Aparece en las colecciones: FCEN - Facultad de Ciencias Exactas y Naturales. UBA

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